WAY too many, but it's a tie between Salt and Sanctuary, FIFA 2012, with an honorable mention of Resident Evil 3.
Phil went into Salt and Sanctuary thinking "Oh, it's easy..." Typical Phil. However, Phil couldn't remember simple hazards and continued to fumble his way through the game, while claiming that he "couldn't remember." hazards that JUST happened a few moments before. My favorite moments is when he looking for a save point, RUNS right past it, and into a boss fight....or simply ignoring signs of a oncoming boss fight by ignoring queues from the game and complaining that the game didn't tell him of an oncoming boss fight. Yes, he rage quit that game and has NEVER gone back to it.
With FIFA 2012, besides him butchering names of football clubs - and this is coming from a Yank for my mentally ill morons on the other side of the pond - he bitched about that he "couldn't play a game." and spend 20 minutes trying to figure out the menu and getting pissed. Once he was able to play a game, he started getting pissy about the controls on beginner. The best part was him gloating about how he was able to "master the controls", he upped the difficulty and got his ass HANDED to him.
There was good salt in FIFA 2012 and Salt and Sanctuary, IMO.
The other one is Resident Evil 3 and the ink ribbon bitching. Still to this VERY day, the idiot saved 33 TIMES and got an F ranking because of it. I honestly thought that was IMPOSSIBLE to get a F ranking in Resident Evil, but Phil being Phil, he finds another rock layer and digs deeper.
There's a ton others of Phil raging, but that's some of my favorites.